Diamond is a leading quantum photonics platform due to its ability to host qubits based on crystal defects such as nitrogen vacancy centres. Fabricating nanophotonic devices from defect-rich diamond, which is central to many quantum sensing technologies, promises to enable enhanced performance and integrability of diamond quantum sensors. Here we demonstrate microdisk cavities fabricated from defect-rich diamond that support optical modes with high quality factor ($Q\sim7\times10^4$ at 1042 nm), and show that they exhibit saturable absorption. Power dependent spectroscopy measurements spanning 979 nm to 1604 nm are used to extract wavelength-dependent absorption coefficients and saturation intensities, which indicate that a hydrogen-related defect is a likely origin of the observed absorption. At 1047 nm, we measure a saturation intensity of 3.3 (1) MW/cm$^2$ and an absorption coefficient of 0.537 (4) cm$^{-1}$. These results provide insight into defect-mediated optical loss in diamond nanophotonics and suggest strategies to harness defect-induced nonlinearities in future diamond photonic devices.
Nanophotonics, an interdisciplinary field merging nanotechnology and photonics, has enabled transformative advancements across diverse sectors including green energy, biomedicine, and optical computing. This review comprehensively examines recent progress in nanophotonic principles and applications, highlighting key innovations in material design, device engineering, and system integration. In renewable energy, nanophotonic allows light-trapping nanostructures and spectral control in perovskite solar cells, concentrating solar power, and thermophotovoltaics. That have significantly enhanced solar conversion efficiencies, approaching theoretical limits. For biosensing, nanophotonic platforms achieve unprecedented sensitivity in detecting biomolecules, pathogens, and pollutants, enabling real-time diagnostics and environmental monitoring. Medical applications leverage tailored light-matter interactions for precision photothermal therapy, image-guided surgery, and early disease detection. Furthermore, nanophotonics underpins next-generation optical neural networks and neuromorphic computing, offering ultra-fast, energy-efficient alternatives to von Neumann architectures. Despite rapid
Rapid progress in precision nanofabrication and atomic design over the past 50 years has ushered in a succession of transformative eras for molding the generation and flow of light. The use of nanoscale and atomic features to design light sources and optical elements-encapsulated by the term nanophotonics-has led to new fundamental science and innovative technologies across the entire electromagnetic spectrum, with substantial emphasis on the microwave to visible regimes. In this review, we pay special attention to the impact and potential of nanophotonics in a relatively exotic yet technologically disruptive regime: high-energy particles such as X-ray photons and free electrons-where nanostructures and atomic design open the doors to unprecedented technologies in quantum science and versatile X-ray sources and optics. As the practical generation of X-rays is intrinsically linked to the existence of energetic free or quasi-free-electrons, our review will also capture related phenomena and technologies that combine free electrons with nanophotonics, including free-electron-driven nanophotonics at other photon energies. In particular, we delve into the demonstration and study of quan
Quantum nanophotonics merges the precision of nanoscale light manipulation with the capabilities of quantum technologies, offering a pathway for enhanced light-matter interaction and compact realization of quantum devices. Here, we show how a recently-demonstrated nonlinear nanophotonic process can be employed to selectively create photonic high-dimensional quantum states (qudits). We utilize the nonlinearity on the surface of the nanophotonic device to dress, through the polarization of the pump field, the near-field modes carrying angular momentum and their superpositions. We then use this approach for the realization of a multilevel quantum key distribution protocol, which doubles the key rate compared to standard schemes. This idea is an important step towards experimental realizations of quantum state generation and manipulation through nonlinearity within nanophotonic platforms, and enables new capabilities for on-chip quantum devices.
Photonics offers unique capabilities for quantum information processing (QIP) such as room-temperature operation, the scalability of nanophotonics, and access to ultrabroad bandwidths and consequently ultrafast operation. Ultrashort-pulse sources of quantum states in nanophotonics are an important building block for achieving scalable ultrafast QIP, however, their demonstrations so far have been sparse. Here, we demonstrate a femtosecond biphoton source in dispersion-engineered periodically poled lithium niobate nanophotonics. We measure 17 THz of bandwidth for the source centered at 2.09 \textmu m, corresponding to a few optical cycles, with a brightness of 8.8 GHz/mW. Our results open new paths towards realization of ultrafast nanophotonic QIP.
Incorporating on-chip light sources directly into nanophotonic waveguides generally requires introducing a different material to the chip than that used for guiding the light, a crucial step that requires dealing with several technical challenges, e.g., atomic lattice mismatch in epitaxial growth between substrate and luminescent materials resulting in strain defects that lower performance. Here we demonstrate that van der Waals materials, such as the 2D semiconductor MoSe2, can easily be transferred onto gold plasmonic nanowaveguides using standard dry visco-elastic polymer transfer techniques. We further show that the photoluminescence from MoSe2 can be injected directly into these on-chip waveguides. Our fabrication methods are compatible with large-scale roll-to-roll manufacturing techniques, highlighting a potential cost-effective and scalable hybrid plasmonic and 2D semiconductor platform for integrated nanophotonics.
Widely-tunable coherent sources are desirable in nanophotonics for a multitude of applications ranging from communications to sensing. The mid-infrared spectral region (wavelengths beyond 2 $μ$m) is particularly important for applications relying on molecular spectroscopy. Among tunable sources, optical parametric oscillators typically offer some of the broadest tuning ranges; however, their implementations in nanophotonics have been limited to narrow tuning ranges and only at visible and near-infrared wavelengths. Here, we surpass these limits in dispersion-engineered periodically-poled lithium niobate nanophotonics and demonstrate ultra-widely tunable optical parametric oscillators. With a pump wavelength near 1 $μ$m, we generate output wavelengths tunable from 1.53 $μ$m to 3.25 $μ$m in a single chip with output powers as high as tens of milliwatts. Our results represent the first octave-spanning tunable source in nanophotonics extending into the mid-infrared which can be useful for numerous integrated photonic applications.
One of the most fundamental quantum states of light is squeezed vacuum, in which noise in one of the quadratures is less than the standard quantum noise limit. Significant progress has been made in the generation of optical squeezed vacuum and its utilization for numerous applications. However, it remains challenging to generate, manipulate, and measure such quantum states in nanophotonics with performances required for a wide range of scalable quantum information systems. Here, we overcome this challenge in lithium niobate nanophotonics by utilizing ultrashort-pulse phase-sensitive amplifiers for both generation and all-optical measurement of squeezed states on the same chip. We generate a squeezed state spanning over more than 25 THz of bandwidth supporting only a few optical cycles, and measure a maximum of 4.9 dB of squeezing ($\sim$11 dB inferred). This level of squeezing surpasses the requirements for a wide range of quantum information systems. Our results on generation and measurement of few-optical-cycle squeezed states in nanophotonics enable a practical path towards scalable quantum information systems with THz clock rates and open opportunities for studying non-classica
When impinging on optical structures or passing in their vicinity, free electrons can spontaneously emit electromagnetic radiation, a phenomenon generally known as cathodoluminescence. Free-electron radiation comes in many guises: Cherenkov, transition, and Smith-Purcell radiation, but also electron scintillation, commonly referred to as incoherent cathodoluminescence. While those effects have been at the heart of many fundamental discoveries and technological developments in high-energy physics in the past century, their recent demonstration in photonic and nanophotonic systems has attracted a lot of attention. Those developments arose from predictions that exploit nanophotonics for novel radiation regimes, now becoming accessible thanks to advances in nanofabrication. In general, the proper design of nanophotonic structures can enable shaping, control, and enhancement of free-electron radiation, for any of the above-mentioned effects. Free-electron radiation in nanophotonics opens the way to promising applications, such as widely-tunable integrated light sources from x-ray to THz frequencies, miniaturized particle accelerators, and highly sensitive high-energy particle detectors.
Transition metal dichalcogenides (TMDs) attract significant attention due to their exceptional optical, excitonic, mechanical, and electronic properties. Nanostructured multilayer TMDs were recently shown to be highly promising for nanophotonic applications, as motivated by their exceptionally high refractive indexes and optical anisotropy. Here, we extend this vision to more sophisticated structures, such as periodic arrays of nanodisks and nanoholes, as well as proof-of-concept waveguides and resonators. We specifically focus on various advanced nanofabrication strategies, including careful selection of resists for electron beam lithography and etching methods. The specific materials studied here include semiconducting WS$_2$, in-plane anisotropic ReS$_2$, and metallic TaSe$_2$, TaS$_2$ and NbSe$_2$. The resulting nanostructures can potentially impact several nanophotonic and optoelectronic areas, including high-index nanophotonics, plasmonics and on-chip optical circuits. The knowledge of TMD material-dependent nanofabrication parameters developed here will help broaden the scope of future applications of these materials in all-TMD nanophotonics.
Recent progress in nanofabrication has led to tremendous technological developments in nanophotonics, which rely on the interaction of light with nanostructured matter. Nanophotonics has experienced a large surge of interest in recent years, from basic research to applied technology. The increased importance of extremely low-energy data processing at ultra-fast speeds has been encouraging the use of light for signal transport and processing. Energy demands and interaction time scales become smaller with the physical size of the nanostructures, hence nanophotonics opens the opportunity of integrating a large number of devices that can generate, control, modulate, sense and process light signals at ultrafast speeds and below femtojoule/bit energy levels. However, losses and diffraction pose fundamental challenges to the fundamental ability of nanophotonic structures to confine light efficiently in smaller and smaller volumes. In this framework, active nanophotonics, which combines the latest advances in nanotechnology with gain materials has become in recent years a vital area of optics research, both from the physics, material science, and engineering standpoint. In this paper, we r
A global trend to miniaturization and multiwavelength performance of nanophotonic devices drives research on novel phenomena, such as bound states in the continuum and Mietronics, as well as the survey for high-refractive index and strongly anisotropic materials and metasurfaces. Hexagonal boron nitride (hBN) is one of promising materials for the future nanophotonics owing to its inherent anisotropy and prospects of high-quality monocrystals growth with atomically flat surface. Here, we present highly accurate optical constants of hBN in the broad wavelength range of 250-1700 nm combining the imaging ellipsometry measurements scanning near-field optical microscopy and first-principle quantum mechanical computations. hBN's high refractive index, up to 2.75 in ultraviolet (UV) and visible range, broadband birefringence of 0.7, and negligible optical losses make it an outstanding material for UV and visible range photonics. Based on our measurement results, we propose and design novel optical elements: handedness-preserving mirrors and subwavelength waveguides with dimensions of 40 nm operating in the visible and UV range, respectively. Remarkably, our results offer unique opportunity
Optical frequency comb is an enabling technology for a multitude of applications from metrology to ranging and communications. The tremendous progress in sources of optical frequency combs has mostly been centered around the near-infrared spectral region while many applications demand sources in the visible and mid-infrared, which have so far been challenging to achieve, especially in nanophotonics. Here, we report frequency combs tunable from visible to mid-infrared on a single chip based on ultra-widely tunable optical parametric oscillators in lithium niobate nanophotonics. Using picosecond-long pump pulses around 1 $μ$m and tuning of the quasi-phase matching, we show sub-picosecond frequency combs tunable beyond an octave extending from 1.5 $μ$m up to 3.3 $μ$m with femtojoule-level thresholds. We utilize the up-conversion of the infrared combs to generate visible frequency combs reaching 620 nm on the same chip. The ultra-broadband tunability and visible-to-mid-infrared spectral coverage of our nanophotonic source can be combined with an on-chip picosecond source as its pump, as well as pulse shortening and spectral broadening mechanisms at its output, all of which are readily
The field of 2D materials-based nanophotonics has been growing at a rapid pace, triggered by the ability to design nanophotonic systems with in situ control, unprecedented degrees of freedom, and to build material heterostructures from bottom up with atomic precision. A wide palette of polaritonic classes have been identified, comprising ultra confined optical fields, even approaching characteristic length scales of a single atom. These advances have been a real boost for the emerging field of quantum nanophotonics, where the quantum mechanical nature of the electrons and-or polaritons and their interactions become relevant. Examples include, quantum nonlocal effects, ultrastrong light matter interactions, Cherenkov radiation, access to forbidden transitions, hydrodynamic effects, single plasmon nonlinearities, polaritonic quantization, topological effects etc. In addition to these intrinsic quantum nanophotonic phenomena, the 2D material system can also be used as a sensitive probe for the quantum properties of the material that carries the nanophotonics modes, or quantum materials in its vicinity. Here, polaritons act as a probe for otherwise invisible excitations, e.g. in superc
In his Comment on our recent paper ``The laws of physics do not prohibit counterfactual communication'', \textit{npj Quantum Information} (2022) 8:60, Popescu argues that the claims of the paper are invalid. Here, we refute his argument, showing that it is based on ignoring the specifics of what we set out to prove (that counterfactual communication is possible \emph{for post-selected particles}, and more specifically in these cases is not prohibited by the weak trace or consistent histories criteria for particle path), followed by an unwarranted simplification of the protocol. Moreover, the Comment's excursion into interpretation is misplaced. Our communication protocol is a precisely defined one that allows two remote parties, albeit rarely, to communicate an arbitrarily long binary message, with arbitrarily high accuracy. This is not a matter of interpretation -- as the concrete example given in our paper in question illustrates. As for our overarching claim that no particles are exchanged in the course of this communication, we have already demonstrated this both theoretically and experimentally, in the postselected case we consider, as per the weak trace and consistent histori
In this Article, we review a novel, rapidly developing field of modern light science named all-dielectric nanophotonics. This branch of nanophotonics is based on the properties of high-index dielectric nanoparticles which allow for controlling both magnetic and electric responses of a nanostructured matter. Here, we discuss optical properties of high-index dielectric nanoparticles, methods of their fabrication, and recent advances in practical applications, including the quantum source emission engineering, Fano resonances in all-dielectric nanoclusters, surface enhanced spectroscopy and sensing, coupled-resonator optical waveguides, metamaterials and metasurfaces, and nonlinear nanophotonics.
Tailoring of electromagnetic spontaneous emission predicted by E. M. Purcell more than 50 years ago has undoubtedly proven to be one of the most important effects in the rich areas of quantum optics and nanophotonics. Although during the past decades the research in this field has been focused on electric dipole emission, the recent progress in nanofabrication and study of magnetic quantum emitters, such as rare-earth ions, has stimulated the investigation of the magnetic side of spontaneous emission. Here, we review the state-of-the-art advances in the field of spontaneous emission enhancement of magnetic dipole quantum emitters with the use of various nanophotonics systems. We provide the general theory describing the Purcell effect of magnetic emitters, overview realizations of specific nanophotonics structures allowing for the enhanced magnetic dipole spontaneous emission, and give an outlook on the challenges in this field, which remain open to future research.
Integrating nanophotonics with electronics promises revolutionary applications, from LiDAR to holographic displays. Although silicon photonics is maturing, realizing active nanophotonics in the ubiquitous bulk CMOS processes remains challenging. We introduce a fabless approach to embed active nanophotonics in bulk CMOS by co-designing the back-end-of-line metal layers for optical functionality. Using a 65nm CMOS process, we create plasmonic liquid crystal modulators with switching speeds 100x faster than commercial technologies. This zero-change nanophotonics method could equip mass-produced chips with optical communications, sensing and imaging. Embedding nanophotonics in the dominant electronics platform democratizes nanofabrication, spawning technologies from chip-scale LiDAR to holographic light-field displays.
Nanophotonics has been an active research field over the past two decades, triggered by the rising interests in exploring new physics and technologies with light at the nanoscale. As the demands of performance and integration level keep increasing, the design and optimization of nanophotonic devices become computationally expensive and time-inefficient. Advanced computational methods and artificial intelligence, especially its subfield of machine learning, have led to revolutionary development in many applications, such as web searches, computer vision, and speech/image recognition. The complex models and algorithms help to exploit the enormous parameter space in a highly efficient way. In this review, we summarize the recent advances on the emerging field where nanophotonics and machine learning blend. We provide an overview of different computational methods, with the focus on deep learning, for the nanophotonic inverse design. The implementation of deep neural networks with photonic platforms is also discussed. This review aims at sketching an illustration of the nanophotonic design with machine learning and giving a perspective on the future tasks.
The reliable measurement and accurate control of the temperature within nanophotonic devices is a key prerequisite for their application in both classical and quantum technologies. Established approaches use sensors that are attached in proximity to the components, which only offers a limited spatial resolution and thus impedes the measurement of local heating effects. Here, we therefore study an alternative temperature sensing technique that is based on measuring the luminescence of erbium emitters directly integrated into nanophotonic silicon waveguides. To cover the entire temperature range from 295 K to 2 K, we investigate two different approaches: The thermal activation of non-radiative decay channels for temperatures above 200 K and the thermal depopulation of spin- and crystal field levels at lower temperatures. The achieved sensitivity is 0.22(4) %/K at room temperature and increases up to 420(50) %/K at approximately 2 K. Within a few-minute measurement interval, we thus achieve a measurement precision that ranges from 0.04(1) K at the lowest studied temperature to 6(1) K at ambient conditions. In the future, the measurement time can be further reduced by optimizing the ex