Aluminum nitride (AlN) is an extremely promising material for integrated photonics because of the combination of strong χ(2) and χ(3) nonlinearities. However, the intrinsic hardness of the material and charging effects during electron beam lithography make AlN nanofabrication a challenging process. Conventional approaches often require multiple hard masks and a metal mask to fabricate nanostructures. In this letter, we report a novel, simple method to fabricate AlN microresonators by using a single layer of silicon nitride mask combined with a thin conductive polymer layer. The conductive layer can be conveniently removed during developing without requiring an additional etching step. We achieve a high etching selectivity of 4:1 between AlN and the mask, enabling mid-infrared photonic device fabrication, as well as high intrinsic quality (Q) factors of up to 1.0 × 10⁶ in AlN microresonators. Furthermore, we demonstrate several nonlinear phenomena within these devices, including frequency comb generation, Raman lasing, third-harmonic generation, and supercontinuum generation.
Spatial modes have found widespread applications in spatial division multiplexing (SDM), sensing, quantum information processing, and on-chip machine learning. The capability to manipulate multiple mode bases will greatly enhance versatility and accelerate the adoption of SDM by remaining agnostic to the specific mode types traversing optical networks. Programmable photonic integrated circuits offer compact and flexible control over spatial modes. In this work, we design and demonstrate a reconfigurable spatial mode generator utilizing a programmable silicon photonic chip. Our architecture leverages orbital angular momentum (OAM) modes as the basis to generate linear polarized (LP) modes and cylindrical vector (CV) modes, providing a scalable solution for spatial mode manipulation across amplitude, phase, and polarization domains. Using a proof-of-concept device, we experimentally generate ten distinct OAM modes and eight LP modes. Furthermore, we numerically analyze experimental errors and propose methods to enhance modal purity and enable effective vector mode generation.
Manipulating intensity, phase and polarisation of the electromagnetic fields on ultrafast timescales is essential for all-optical switching, optical information processing and development of novel time-variant media. Noble metal based plasmonics has provided numerous platforms for optical switching and control, enabled by strong local field enhancement, artificially engineered dispersion and strong Kerr-type free-electron nonlinearities. However, achieving precise control over switching times and spectral response remains challenging, often limited by hot-electron gas relaxation on picosecond timescales and by the intrinsic band structure of the materials. Here, we experimentally demonstrate a strong and tunable nonlinearity in a metamaterial-on-a-mirror geometry, controlled by the wavelength of excitation, which imprints a specific, non-uniform hot-electron population distribution, driving targeted electron and lattice dynamics. The synergistic exchange of electromagnetic, electronic and mechanical energies enables reflection changes on sub-300 fs timescales in selected spectral ranges, surpassing the limitations imposed by the inherent material response of metamaterial constituents. The observed effect-present in reflection due to leaky guided modes of the metamaterial, but absent in transmission-is highly spectrally selective and sensitive to polarisation of light, opening a pathway to tailoring switching rates through the choice of operating wavelength and nanostructure design. The ability to manipulate temporal, spectral, and mechanical aspects of light-matter interactions underscores new opportunities for nonlinear optical applications where polarisation diversity, spectral selectivity, and ultrafast modulation are important.
Mid-infrared molecular sensing offers molecule-specific vibrational fingerprints, yet practical implementation with nanophotonic platforms is challenged by system complexity and strong signal damping in aqueous environments. Dielectric metasurfaces overcome ohmic losses and local heating constraints of metallic resonators and can support high-quality-factor resonances with spectral selectivity, suitable for image-based spectrometer-less sensing. However, their spatially extended near-fields typically render them susceptible to environmental absorption, preventing operation in water. We demonstrate a compact dielectric perfect-absorber metasurface combining C4-symmetric quasi-bound states in the continuum (qBICs) with a dual-gradient architecture. The C4-symmetric unit cells ensure polarization-independent resonances, enabling efficient utilization of incident light under arbitrary polarization states. The gradient architecture independently controls radiative loss and resonance wavelength, allowing distinct coupling regimes within one metasurface while achieving high absorbance (>0.8). We demonstrate poly(methyl methacrylate) sensing in air with ~20% absorbance envelope modulation under arbitrary polarization. Furthermore, we introduce a sensing configuration utilizing a 700 nm residual thin-water film that preserves qBIC (absorbance ~0.5) near the prominent water absorption peak. This enables the first demonstration of dielectric metasurface-based mid-infrared molecular sensing under a water background, achieving >30% absorbance envelope modulation. This platform extends the utility of dielectric metasurfaces to aqueous environments and supports versatile, spectrometer-less sensing schemes.
Spin-active colour centres in 4H silicon carbide are promising candidates as building blocks for quantum information applications. To increase the photon count rate of the emitters at low temperatures, the colour centres must be integrated into nanophotonic structures and characterised under cryogenic conditions. Here, we design and fabricate waveguide structures attached with an efficient Dinosaur photonic crystal reflector at one side. The devices show broadband reflection over a range of 60 THz with a peak reflectance above 80 %. Additionally, colour centres were integrated into these structures and characterised at cryogenic conditions. The emission was collected by a tapered-waveguide-tapered-fibre interface. Although the spectral stability of the emitters must be further improved for high excitation powers, the saturation intensity in standard PLE measurements is I s,LT = (103.8 ± 4.2) kcps. The count rate can be further improved to about 125 kcps with a charge-resonance check measurement scheme. To highlight the relevance of our devices, we theoretically show that these count rates enable optical single-shot readout with a fidelity exceeding 98%.
Second-order nonlinear optical processes are fundamental to photonics, spectroscopy, and information technologies, with material platforms playing a pivotal role in advancing these applications. Here, we demonstrate the exceptional nonlinear optical properties of the van der Waals crystal 3R-MoS2, a rhombohedral polymorph exhibiting high second-order optical susceptibility (χ (2)) and remarkable second-harmonic generation (SHG) capabilities. By designing high quality factor resonances in 3R-MoS2 metasurfaces supporting quasi-bound states in the continuum (qBIC), we first demonstrate SHG efficiency enhancement exceeding 102. Additionally, by using degenerate pump-probe spectroscopy, we harness the C 3v system's symmetry to realize ultrafast SHG polarization switching with near-unity modulation depth. The operation speeds are limited only by the excitation pulse duration, allowing its characterization via the nonlinear autocorrelation function. These findings establish 3R-MoS2 as a transformative platform for nanoscale nonlinear optics, offering large conversion efficiencies and ultrafast response times for advanced pulse measurement devices, integrated photonics, and quantum technologies.
We introduce a novel material for integrated photonics and investigate aluminum gallium nitride (AlGaN) on aluminum nitride (AlN) templates as a platform for developing reconfigurable and on-chip nonlinear optical devices. AlGaN combines compatibility with standard photonic fabrication technologies and high electro-optic modulation capabilities with low loss over a broad spectral range, from UVC to long-wave infrared, making it a viable material for complex photonic applications. In this work, we design and grow AlGaN/AlN heterostructures and integrate several photonic components. In particular, we fabricate edge couplers, low-loss waveguides, directional couplers, and tunable high-quality factor ring resonators. These devices will enable nonlinear light-matter interaction and quantum functionality. The comprehensive platform we present in this work paves the way for photon-pair generation applications, on-chip quantum frequency conversion, and fast electro-optic modulation for switching and routing classical and quantum light fields.
Manipulating the phase of an optical wave over time and frequency gives full control to the user to implement a wide variety of energy preserving transformations directly in the analogue optical domain. These can be achieved using widely available linear mechanisms, such as temporal phase modulation and spectral phase filtering. The techniques based on these linear optical wave energy redistribution (OWER) methods are inherently energy efficient and have significant speed and bandwidth advantages over digital signal processing. We describe several recent OWER methods for optical signal processing, including denoising passive amplification, real-time spectrogram analysis, passive logic computing, and more. These functionalities are relevant whenever the signal is found on a classical or quantum optical wave, or could be upconverted from radio frequencies or microwaves, and they are of interest for a wide range of applications in telecommunications, sensing, metrology, biomedical imaging, and astronomy. The energy preservation of these methods makes them particularly interesting for quantum optics applications. Furthermore, many of the individual components have been demonstrated on-chip, enabling miniaturization for applications where size and weight are a main constraint.
The interrelationship between localization, quantum transport, and disorder has remained a fascinating focus in scientific research. Traditionally, it has been widely accepted in the physics community that in one-dimensional systems, as disorder increases, localization intensifies, triggering a metal-insulator transition. However, a recent theoretical investigation [Phys. Rev. Lett. 126, 106803] has revealed that the interplay between dimerization and disorder leads to a reentrant localization transition, constituting a remarkable theoretical advancement in the field. Here, we present the first experimental observation of reentrant localization using an experimentally friendly model, a photonic SSH lattice with random-dimer disorder, achieved by incrementally adjusting synthetic potentials. In the presence of correlated on-site potentials, certain eigenstates exhibit extended behavior following the localization transition as the disorder continues to increase. We directly probe the wave function in disordered lattices by exciting specific lattice sites and recording the light distribution. This reentrant phenomenon is further verified by observing an anomalous peak in the normalized participation ratio. Our study enriches the understanding of transport in disordered mediums and accentuates the substantial potential of integrated photonics for the simulation of intricate condensed matter physics phenomena.
Neuromorphic (brain-inspired) photonics accelerates AI1 with high-speed, energy-efficient solutions for RF communication2, image processing3,4, and fast matrix multiplication5,6. However, integrated neuromorphic photonic hardware faces size constraints that limit network complexity. Recent advances in photonic quantum hardware7 and performant trainable quantum circuits8 offer a path to more scalable photonic neural networks. Here, we show that a combination of classical network layers with trainable continuous variable quantum circuits yields hybrid networks with improved trainability and accuracy. On a classification task, these hybrid networks match the performance of classical networks nearly twice their size. These performance benefits remain even when evaluated at state-of-the-art bit precisions for classical and quantum hardware. Finally, we outline available hardware and a roadmap to hybrid architectures. These hybrid quantum-classical networks demonstrate a unique route to enhance the computational capacity of integrated photonic neural networks without increasing the network size.
Quantum state teleportation represents a pillar of quantum information and a milestone on the roadmap towards quantum networks with a large number of nodes. Successful photonic demonstrations of this protocol have been carried out employing different qubit encodings. However, demonstrations in the Fock basis encoding are challenging, due to the impossibility of generating a coherent superposition of vacuum-one photon states on a single mode with linear optics. Indeed, previous realizations only allowed the teleportation of dual-rail entangled states, by exploiting ancillary electromagnetic modes. Here, instead, we enable the quantum teleportation of pure vacuum-one-photon qubits encoded in a single spatial mode, by exploiting coherent control of a resonantly excited semiconductor quantum dot in a micro-cavity. Within our setup, we can both teleport genuine single-rail vacuum-one-photon qubits and perform entanglement swapping. Our results may disclose new quantum information processing potentialities for this encoding, whose manipulation is achievable via quantum dot single-photon sources.
Nano-optomechanical sensors exploit light confinement at the nanoscale to enable very precise measurements of displacement, force, acceleration, and mass. Their application is hampered by the complex optical set-ups or packaging schemes required to couple light to and from the nano-optomechanical resonator. In this work, we present a fiber-coupled nano-optomechanical sensor that requires no coupling optics. This is achieved by directly placing a nano-optomechanical structure, a double membrane photonic crystal (DM-PhC), on the facet of a fiber, using a simple and scalable wafer-to-fiber transfer method. The device is probed in reflection and has a resonance at telecom wavelengths with a relatively broad spectral width of 3-10 nm, which is advantageous for a simple read-out and achieves a displacement imprecision of 10 fm / Hz . Using resonant driving and a ringdown measurement, we can induce and monitor mechanical oscillations with an nm-scale amplitude via the fiber, which allows for tracking the mechanical resonant frequency and the mechanical linewidth with imprecisions of 79 and 12 Hz, respectively, at integration times of 4.5 s. We further demonstrate the application of this fiber-tip sensor to the measurement of pressure, using the effect of collisional damping on the mechanical linewidth, leading to the imprecision of 9 × 10 - 4 mbar with an integration time of 290 s. This combination of optomechanics and fiber-tip sensing may open the way to a new generation of fiber sensors with unprecedented functionality, ultrasmall footprint, and low-cost readout.
The nitrogen-vacancy center in diamond is an attractive resource for the generation of remote entangled states owing to its optically addressable and long-lived electronic spin. However, its low native fraction of coherent photon emission, ~3%, undermines the achievable spin-photon entanglement rates. Here, we couple a nitrogen-vacancy center with a narrow extrinsically-broadened linewidth (159 MHz), hosted in a micron-thin membrane, to an open microcavity. The resulting Purcell factor of ~1.8 increases the zero-phonon line fraction to over 44%. Operation in the Purcell regime, together with an efficient collection of the zero-phonon-line photons, allows resonance fluorescence to be detected for the first time without any temporal filtering. We achieve a >10 signal-to-laser background ratio. This selective enhancement of the center's zero-phonon transitions could increase spin-spin entanglement success probabilities beyond an order of magnitude compared to state-of-the-art implementations, and enable powerful quantum optics techniques such as wave-packet shaping or all-optical spin manipulation.
Sunlight is widely seen as one of the most abundant forms of renewable energy, with photovoltaic cells based on pn junctions being the most commonly used platform attempting to harness it. Unlike in conventional photovoltaic cells, the bulk photovoltaic effect (BPVE) allows for the generation of photocurrent and photovoltage in a single material without the need to engineer a pn junction and create a built-in electric field, thus offering a solution that can potentially exceed the Shockley-Queisser efficiency limit. However, it requires a material with no inversion symmetry and is therefore absent in centrosymmetric materials. Here, we demonstrate that breaking the inversion symmetry by structural disorder can induce BPVE in ultrathin PtSe2, a centrosymmetric semiconducting van der Waals material. Homogenous illumination of defective PtSe2 by linearly and circularly polarized light results in a photoresponse termed as linear photogalvanic effect (LPGE) and circular photogalvanic effect (CPGE), which is mostly absent in the pristine crystal. First-principles calculations reveal that LPGE originates from Se vacancies that act as asymmetric scattering centers for the photo-generated electron-hole pairs. Our work emphasizes the importance of defects to induce photovoltaic functionality in centrosymmetric materials and shows how the range of materials suitable for light sensing and energy-harvesting applications can be extended.
Diamond is a leading quantum photonics platform due to its ability to host qubits based on crystal defects such as nitrogen-vacancy centres. Fabricating nanophotonic devices from defect-rich diamond, which underpins many quantum sensing technologies, promises enhanced performance and integrability of diamond quantum sensors. Here we demonstrate microdisk cavities fabricated from defect-rich diamond that support optical modes with high quality factor (${Q}\sim7\times10^4$ at $1042\,$nm) and show that they exhibit saturable absorption. Power-dependent spectroscopy measurements spanning 979$\,$nm to 1604$\,$nm are used to observe intensity-dependent cavity loss and extract wavelength-dependent absorption coefficients and saturation intensities. At 1047$\,$nm, we observe saturation and measure a saturation intensity of $2.1\,(8)\,$MW/cm$^2$ and an absorption coefficient of $0.53\,(2)\,$cm$^{-1}$. These results provide insight into defect-mediated optical loss in diamond nanophotonics and suggest strategies to harness defect-induced nonlinearities in future diamond photonic devices.
Nanophotonics, an interdisciplinary field merging nanotechnology and photonics, has enabled transformative advancements across diverse sectors including green energy, biomedicine, and optical computing. This review comprehensively examines recent progress in nanophotonic principles and applications, highlighting key innovations in material design, device engineering, and system integration. In renewable energy, nanophotonic allows light-trapping nanostructures and spectral control in perovskite solar cells, concentrating solar power, and thermophotovoltaics. That have significantly enhanced solar conversion efficiencies, approaching theoretical limits. For biosensing, nanophotonic platforms achieve unprecedented sensitivity in detecting biomolecules, pathogens, and pollutants, enabling real-time diagnostics and environmental monitoring. Medical applications leverage tailored light-matter interactions for precision photothermal therapy, image-guided surgery, and early disease detection. Furthermore, nanophotonics underpins next-generation optical neural networks and neuromorphic computing, offering ultra-fast, energy-efficient alternatives to von Neumann architectures. Despite rapid
Rapid progress in precision nanofabrication and atomic design over the past 50 years has ushered in a succession of transformative eras for molding the generation and flow of light. The use of nanoscale and atomic features to design light sources and optical elements-encapsulated by the term nanophotonics-has led to new fundamental science and innovative technologies across the entire electromagnetic spectrum, with substantial emphasis on the microwave to visible regimes. In this review, we pay special attention to the impact and potential of nanophotonics in a relatively exotic yet technologically disruptive regime: high-energy particles such as X-ray photons and free electrons-where nanostructures and atomic design open the doors to unprecedented technologies in quantum science and versatile X-ray sources and optics. As the practical generation of X-rays is intrinsically linked to the existence of energetic free or quasi-free-electrons, our review will also capture related phenomena and technologies that combine free electrons with nanophotonics, including free-electron-driven nanophotonics at other photon energies. In particular, we delve into the demonstration and study of quan
Quantum nanophotonics merges the precision of nanoscale light manipulation with the capabilities of quantum technologies, offering a pathway for enhanced light-matter interaction and compact realization of quantum devices. Here, we show how a recently-demonstrated nonlinear nanophotonic process can be employed to selectively create photonic high-dimensional quantum states (qudits). We utilize the nonlinearity on the surface of the nanophotonic device to dress, through the polarization of the pump field, the near-field modes carrying angular momentum and their superpositions. We then use this approach for the realization of a multilevel quantum key distribution protocol, which doubles the key rate compared to standard schemes. This idea is an important step towards experimental realizations of quantum state generation and manipulation through nonlinearity within nanophotonic platforms, and enables new capabilities for on-chip quantum devices.
Photonics offers unique capabilities for quantum information processing (QIP) such as room-temperature operation, the scalability of nanophotonics, and access to ultrabroad bandwidths and consequently ultrafast operation. Ultrashort-pulse sources of quantum states in nanophotonics are an important building block for achieving scalable ultrafast QIP, however, their demonstrations so far have been sparse. Here, we demonstrate a femtosecond biphoton source in dispersion-engineered periodically poled lithium niobate nanophotonics. We measure 17 THz of bandwidth for the source centered at 2.09 \textmu m, corresponding to a few optical cycles, with a brightness of 8.8 GHz/mW. Our results open new paths towards realization of ultrafast nanophotonic QIP.
Incorporating on-chip light sources directly into nanophotonic waveguides generally requires introducing a different material to the chip than that used for guiding the light, a crucial step that requires dealing with several technical challenges, e.g., atomic lattice mismatch in epitaxial growth between substrate and luminescent materials resulting in strain defects that lower performance. Here we demonstrate that van der Waals materials, such as the 2D semiconductor MoSe2, can easily be transferred onto gold plasmonic nanowaveguides using standard dry visco-elastic polymer transfer techniques. We further show that the photoluminescence from MoSe2 can be injected directly into these on-chip waveguides. Our fabrication methods are compatible with large-scale roll-to-roll manufacturing techniques, highlighting a potential cost-effective and scalable hybrid plasmonic and 2D semiconductor platform for integrated nanophotonics.