搜索结果：sub-1s

The advent of novel free-electron laser sources enabling time-resolved x-ray photoelectron spectroscopy (tr-XPS) provides a unique opportunity to monitor local chemical environments in real time by measuring sub-eV shifts in core-electron binding energies. These shifts reflect the interplay between electronic excitation and nuclear motion, an interplay that remains largely unexplored. In our combined theoretical and experimental study of fluoropyridine (C$_5$H$_4$FN), we investigate this link by monitoring the evolving chemical environment at the N and F atomic sites as the photoexcited $S_1$ state relaxes to the ground state via a conical intersection. We find that the F site responds primarily to vibrational relaxation, showing minimal sensitivity to the electronic excited state. In contrast, excitation to $S_1$ induces a measurable energy shift at the N site and significantly enhances its sensitivity to local vibrations within the ring. This behavior arises from a photoinduced redistribution of charge, which also increases the Coulomb interaction between the 1s electron at the N atom and the atomic partial charge at an adjacent C atom. This insight opens new avenues for explorin

The non-perturbative evaluation of multipolar cross sections is essential for probing atomic and molecular responses to spatially inhomogeneous electric fields characteristic of nanoscale environments where the conventional dipole approximation breaks down. Taking the hydrogen atom as an analytical and numerical benchmark, we map in real time quadrupole interactions driven by instantaneous electric field gradients. Our study explores two distinct interaction regimes. Under a uniform field, quadrupolar responses are activated by multi-step dipole transitions, responsible for sub-1~eV excited-state absorption. Conversely, under pure spatial gradients, the weak-field response is dominated by the single-photon $1s \to 3d$ quadrupole resonance at 12.1~eV, while strong gradients induce low-energy stimulated emission via transiently driven coherent populations. This dynamical analysis is complemented by a rigorous evaluation of the symmetry aspects of the quadrupole response and the applied electric field. This methodology establishes the theoretical and computational foundation for future non-perturbative multipole simulations of molecules and nanostructures in the near-field regime.

Deploying humanoid robots in real-world settings is fundamentally challenging, as it demands tight integration of perception, locomotion, and manipulation under partial-information observations and dynamically changing environments. As well as transitioning robustly between sub-tasks of different types. Towards addressing these challenges, we propose a novel task - EgoActing, which requires directly grounding high-level instructions into various, precise, spatially aware humanoid actions. We further instantiate this task by introducing EgoActor, a unified and scalable vision-language model (VLM) that can predict locomotion primitives (e.g., walk, turn, move sideways, change height), head movements, manipulation commands, and human-robot interactions to coordinate perception and execution in real-time. We leverage broad supervision over egocentric RGB-only data from real-world demonstrations, spatial reasoning question-answering, and simulated environment demonstrations, enabling EgoActor to make robust, context-aware decisions and perform fluent action inference (under 1s) with both 8B and 4B parameter models. Extensive evaluations in both simulated and real-world environments demo

Reddened Type-1 quasars offer a unique window into the structure and evolution of active galactic nuclei (AGN), yet their physical origin and the source of their reddening remain uncertain. Optical surveys often miss these dust-obscured objects, resulting in an incomplete view of the quasar population. In this work, we construct a sample of 6,600 Type-1 quasars at redshifts $0.5 \leq z \leq 1.2$ by combining deep optical imaging from HSC with mid-infrared photometry from WISE, enabling a more complete selection that is not biased against reddened objects. We perform detailed SED modeling using the CIGALE code, enhanced by synthetic photometry derived from SDSS spectra to better constrain the optical continuum. We classify quasars into blue and reddened Type-1 populations based on their continuum slopes and compare their SEDs and emission line properties. As expected from this definition, reddened Type-1 AGN show higher dust extinction, with a median $A_V = 0.60^{+0.32}_{-0.19}$ mag, compared to $A_V = 0.06^{+0.10}_{-0.03}$ mag for blue objects. But they also exhibit smaller torus half-opening angles, with a median of $25.7^{+10.1}_{-8.7}$ deg, compared to $33.3^{+11.1}_{-5.9}$ deg

The ability to control absorption by modifying the polarization of light presents an exciting opportunity to experimentally determine the orbital alignment of absorption features. Here, attosecond extreme ultraviolet (XUV) transient absorption spectroscopy is used to investigate the polarization dependence of core exciton dynamics in LiF thin films at the Li+ K edge. XUV pulses excite electrons from the Li 1s core level into the conduction band, allowing for the formation of a p-orbital-like core exciton, aligned along the XUV light polarization axis. A sub-5 fs near-infrared (NIR) probe pulse then arrives at variable time delays, perturbing the XUV-excited states and allowing the coherence decay of the core exciton to be mapped. The coherence lifetimes are found to be ~2.4 +- 0.4 fs, which is attributed to a phonon-mediated dephasing mechanism as in previous core exciton studies. The differential absorption features are also shown to be sensitive to the relative polarization of the XUV and NIR fields. The parallel NIR probe induces couplings between the initial XUV-excited p-like bright exciton and s-like dark excitons. When crossed pump and probe polarizations are used, the coupl

The universality of free fall, a cornerstone of Einstein's theory of gravity, has so far only been tested with neutral composite states of first-generation Standard Model (SM) particles, such as atoms or neutrons, and, most recently, antihydrogen. Extending these gravitational measurements to other sectors of the SM requires the formation of neutral bound states using higher-generation, unstable particles. Muonium, the bound state of an antimuon ($μ^+$) and an electron ($e^-$), offers the possibility to probe gravity with second-generation (anti)leptons, in the absence of the strong interaction. However, the short $μ^+$ lifetime ($τ_μ\approx 2.2~μ$s) and the existing diffuse thermal muonium sources rendered such measurements unfeasible. Here, we report the synthesis of a high-brightness muonium beam, extracted from a thin layer of superfluid helium by exploiting its chemical potential and unique transport properties. The mean longitudinal velocity (${v}\approx 2180~\rm{m/s}$) and narrow distribution (${Δv}< 150 ~\rm{m/s}$) of the atoms characterise a superthermal beam, while yields are similar to the highest intensity diffuse sources. This new beam is expected to enable muonium

Dusty star-forming galaxies (DSFGs) dominate the far-infrared and sub-millimetre number counts, but single-dish surveys suffer from poor angular resolution, complicating mult-wavelength counterpart identification. Prior-driven deblending techniques require extensive fine-tuning and struggle to process large fields. This work aims to develop a fast, reliable deep-learning based deconvolution and denoising super-resolution (SR) technique. We employ a transformer neural network to improve the resolution of Herschel/SPIRE 500 $μ$m observations by a factor 4.5, using Spitzer/MIPS 24$μ$m and Herschel/SPIRE 250, 350, 500$μ$m images. Trained on SIDES and SHARK simulations, we injected instrumental noise into the input simulated images, while keeping the target images noise-free to enhance de-noising capabilities of our method. We evaluated the performance on simulated test sets and real JCMT/SCUBA-2 450 $μ$m observations in the COSMOS field which have superior resolution compared to Herschel. Our SR method achieves an inference time of $1s/deg^2$ on consumer GPUs, much faster than traditional deblending techniques. Using the simulation test sets, we show that fluxes of the extracted source

We present an optical variability analysis and comparison of the samples of Seyfert 1 and 2 galaxies, selected from the \textit{Swift} 9-month BAT catalog, using the light curves from Transiting Exoplanet Survey Satellite (TESS) and All-Sky Automated Survey for SuperNovae (ASAS-SN). We measured the normalized excess variance of TESS and ASAS-SN light curves for each target and performed a Kolmogorov-Smirnov test between the two samples, where our results showed significant differences. This is consistent with predictions from the unification model, where Seyfert 2s are obscured by the larger scale dust torus and their variability is suppressed. This variability difference is independent of the luminosity, Eddington ratio, or black hole mass, further supporting geometrical unification models. We searched the dependence of the normalized excess variance of Seyfert 1s on absolute magnitudes, Eddington ratio, and black hole mass, where our results are consistent with relations found in the literature. Finally, a small sub-sample of changing-look AGNs that transitioned during the time frame of the ASAS-SN light curves, with their variability amplitudes changing according to the classifi

Compact symmetric objects (CSOs) are a unique class of jetted active galactic nuclei (AGN) defined by sub-kpc radio emission, showing radio structure on both sides of the central engine. CSOs tend to exhibit little to no relativistic beaming, thereby allowing us to determine their physical characteristics, such as the magnetic field strength and particle energy density. Selected with a literature search, we describe VLBI observations, imaging, and analyses of 167 CSO candidates. We identified 65 new bona fide CSOs, thus almost doubling the number of known bona fide CSOs to 144. With our greater breadth of sources, we confirm that edge-dimmed CSOs (CSO-1s) may represent a more diverse population than originally expected. We highlight a number of CSOs with complex morphologies, including candidates for supermassive binary black holes (SBBHs) and CSOs that appear to have morphologies akin to wide-angle tail (WAT) galaxies, which could perhaps indicate that some CSOs are experiencing a galactic merger.

We propose a concept for a cryogenic source of atomic tritium at sub-Kelvin temperatures and energies suitable for magnetic trapping. The source is based on the dissociation of solid molecular T2 films below 1 K by electrons from a pulsed RF discharge, a technique recently demonstrated for atomic hydrogen, combined with buffer-gas cooling and magnetic confinement. We analyze the key processes limiting the source performance, adsorption, spin exchange and recombination, and show that atomic tritium fluxes exceeding 1e15 1/s at kinetic energies of 100 mK can be achieved at the entrance to the magnetic trap. Such a source would enable Doppler-free two-photon 1S-2S spectroscopy in atomic tritium for high-precision measurements of the triton charge radius, providing a crucial benchmark for bound-state QED and improving the comparison between electronic, muonic, and scattering determinations of nuclear sizes in light systems. Beyond spectroscopy, an atomic tritium source avoids molecular final state broadening in the beta decay and is therefore necessary for next generation neutrino mass measurements; combined with detector technologies such as sub-eV resolution quantum sensors or cyclot

Jaccard Similarity is a very common proximity measurement used to compute the similarity between two asymmetric binary vectors. Jaccard Similarity is the ratio between the 1s (Intersection of two vectors) to 1s (Union of two vectors). This paper introduces a quantum algorithm for finding the Jaccard Similarity 1s, in the Intersection and Union of two binary vectors. There are two sub-algorithms one for each. Measuring the register for respective algorithm gives count of number of 1 s in binary format. Implementation on IBM composer is also included.

Since the invention of the laser nonlinear effects such as filamentation, Rabi-cycling and collective emission have been explored in the optical regime leading to a wide range of scientific and industrial applications. X-ray free electron lasers (XFELs) have led to the extension of many optical techniques to X-rays for their advantages of angstrom scale spatial resolution and elemental specificity. One such example is XFEL driven population inversion of 1s core hole states resulting in inner-shell K$α$ (2p to 1s) X-ray lasing in elements ranging from neon to copper, which has been utilized for nonlinear spectroscopy and development of next generation X-ray laser sources. Here we show that strong lasing effects, similar to those observed in the optical regime, can occur at 1.5 to 2.1 angstrom wavelengths during high intensity (> ${10^{19}}$ W/cm${^{2}}$) XFEL driven inner-shell lasing and superfluorescence of copper and manganese. Depending on the temporal substructure of the XFEL pump pulses(containing ${~10^{6}}$ - ${10^{8}}$ photons) i, the resulting inner-shell X-ray laser pulses can exhibit strong spatial inhomogeneities as well as spectral splitting, inhomogeneities and bro

The Canadian Hydrogen Intensity Mapping Experiment Fast Radio Burst (CHIME/FRB) Project has a new VLBI Outrigger at the Green Bank Observatory (GBO), which forms a 3300km baseline with CHIME operating at 400-800MHz. Using 100ms long full-array baseband "snapshots" collected commensally during FRB and pulsar triggers, we perform a shallow, wide-area VLBI survey covering a significant fraction of the Northern sky targeted at the positions of compact sources from the Radio Fundamental Catalog. In addition, our survey contains calibrators detected from two 1s long trial baseband snapshots for a deeper survey with CHIME and GBO. In this paper, we present the largest catalog of compact calibrators suitable for 30-milliarcsecond-scale VLBI observations at sub-GHz frequencies to date. Our catalog consists of 200 total calibrators in the Northern Hemisphere that are compact on 30-milliarcsecond scales with fluxes above 100mJy. This calibrator grid will enable the precise localization of hundreds of FRBs a year with CHIME/FRB-Outriggers.

JWST, despite not being designed to observe astrophysical phenomena that vary on rapid time scales, can be an unparalleled tool for such studies. If timing systematics can be controlled, JWST will be able to open up the sub-second infrared timescale regime. Rapid time-domain studies, such as lag measurements in accreting compact objects and Solar System stellar occultations, require both precise inter-frame timing and knowing when a time series begins to an absolute accuracy significantly below 1s. In this work we present two long-duration observations of the deeply eclipsing double white dwarf system ZTF J153932.16+502738.8, which we use as a natural timing calibrator to measure the absolute timing accuracy of JWST's clock. From our two epochs, we measure an average clock accuracy of $0.12\pm0.06$s, implying that JWST can be used for sub-second time-resolution studies down to the $\sim100$ms level, a factor $\sim5$ improvement upon the pre-launch clock accuracy requirement. We also find an asymmetric eclipse profile in the F322W2 band, which we suggest has a physical origin.

Supporting ultra-high data rates and flexible reconfigurability, Terahertz (THz) mesh networks are attractive for next-generation wireless backhaul systems that empower the integrated access and backhaul (IAB). In THz mesh backhaul networks, the efficient cross-layer routing and long-term resource allocation is yet an open problem due to dynamic traffic demands as well as possible link failures caused by the high directivity and high non-line-of-sight (NLoS) path loss of THz spectrum. In addition, unpredictable data traffic and the mixed integer programming property with the NP-hard nature further challenge the effective routing and long-term resource allocation design. In this paper, a deep reinforcement learning (DRL) based cross-layer design in THz mesh backhaul networks (DEFLECT) is proposed, by considering dynamic traffic demands and possible sudden link failures. In DEFLECT, a heuristic routing metric is first devised to facilitate resource efficiency (RE) enhancement regarding energy and sub-array usages. Furthermore, a DRL based resource allocation algorithm is developed to realize long-term RE maximization and fast recovery from broken links. Specifically in the DRL method

The ultrafast formation of strongly bound excitons in two-dimensional semiconductors provide a rich platform for studying fundamental physics as well as developing novel optoelectronic technologies. While extensive research has explored the excitonic coherence, many-body interactions, and nonlinear optical properties, the potential to study these phenomena by directly controlling their coherent polarization dynamics has not been fully realized. In this work, we use a sub-10fs pulse shaper to study how temporal control of coherent exciton polarization affects the generation of four-wave mixing in monolayer WSe2 under ambient conditions. By tailoring multiphoton pathway interference, we tune the nonlinear response from destructive to constructive interference, resulting in a 2.6-fold enhancement over the four-wave mixing generated by a transform-limited pulse. This demonstrates a general method for nonlinear enhancement by shaping the pulse to counteract the temporal dispersion experienced during resonant light-matter interactions. Our method allows us to excite both 1s and 2s states, showcasing a selective control over the resonant state that produces nonlinearity. By comparing our

We analyse a sample of 21 `bare' Seyfert~1 Active Galactic Nuclei (AGNs), a sub-class of Seyfert~1s, with intrinsic absorption $\mathrm{N_{H}} \sim 10^{20}~ \mathrm{cm}^{-2}$, in the local universe (z $<$ 0.2) using {\it XMM-Newton} and {\it Swift}/XRT observations. The luminosities of the primary continuum, the X-ray emission in the 3 to 10 keV energy range and the soft-excess, the excess emission that appears above the low-energy extrapolation of the power-law fit of 3 to 10 keV X-ray spectra, are calculated. Our spectral analysis reveals that the long-term intrinsic luminosities of the soft-excess and the primary continuum are tightly correlated $(L_{PC}\propto L_{SE}^{1.1\pm0.04})$. We also found that the luminosities are correlated for each source. This result suggests that both the primary continuum and soft excess emissions exhibit a dependency on the accretion rate in a similar way.

The triplet contribution is computed to the 1 and 2 $^1S^\text{e}_0$ states of the He atom, to the $1\ ^1S^\text{e}_0$ state of the Li$^+$ and Be${^{2+}}$ ions, and to the $X\ ^1Σ_\text{g}^+$ ground state of the H$_2$ molecule by extensive use of double-group symmetry (equivalent to $LS$ coupling for the atomic systems) during the course of the variational solution of the no-pair Dirac-Coulomb-Breit wave equation. The no-pair Dirac-Coulomb-Breit energies are converged within a sub-parts-per-billion relative precision using an explicitly correlated Gaussian basis optimized to the non-relativistic energies. The $α$ fine-structure constant dependence of the triplet sector contribution to the variational energy is $α^4E_\text{h}$ at leading order, in agreement with the formal perturbation theory result available from the literature.

Wide-band-gap insulators such as NiO offer the exciting prospect of coherently manipulating electronic correlations with strong optical fields. Contrary to metals where rapid dephasing of optical excitation via electronic processes occurs, the sub-gap excitation in charge-transfer insulators has been shown to couple to low-energy bosonic excitations. However, it is currently unknown if the bosonic dressing field is composed of phonons or magnons. Here we use the prototypical charge-transfer insulator NiO to demonstrate that 1.5 eV sub-gap optical excitation leads to a renormalised NiO band-gap in combination with a significant reduction of the antiferromagnetic order. We employ element-specific X-ray reflectivity at the FLASH free-electron laser to demonstrate the reduction of the upper band-edge at the O 1s-2p core-valence resonance (K-edge) whereas the antiferromagnetic order is probed via X-ray magnetic linear dichroism (XMLD) at the Ni 2p-3d resonance (L2-edge). Comparing the transient XMLD spectral line shape to ground-state measurements allows us to extract a spin temperature rise of 65 +/- 5 K for time delays longer than 400 fs while at earlier times a non-equilibrium spin s