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The dataset contains all raw data and python scripts (.py) for creating the figures Fig. 3 - Fig. 6 in the main manuscript "Reliability challenges for resistive random-access memory-based parallel logic computing" and the Fig. S3 in the corresponding supplementary information. The data is structured in subfolders according to the individual figures. Please note that Fig.3 and Fig. 4 b-d of the main manuscript operate on the same data. Therefore, the raw data files from subfolder Fig.3 have to be copied in the Fig. 4 subfolder prior to execution.
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We discuss some claims that certain UCOMP devices can perform hypercomputation (compute Turing-uncomputable functions) or perform super-Turing computation (solve NP-complete problems in polynomial time). We discover that all these claims rely on the provision of one or more unphysical resources.
The transistor celebrated its 75 <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">th</sup> birthday in 2022. The continued scaling of the transistor defined by Moore’s Law continues, albeit at a slower pace. Meanwhile, computing demands and energy consumption required by modern artificial intelligence (AI) algorithms have skyrocketed. As an alternative to scaling transistors for general-purpose computing, the integration of transistors with unconventional technologies has emerged as a promising path for domain-specific computing. In this article, we provide a full-stack review of probabilistic computing with p-bits as a representative example of the energy-efficient and domain-specific computing movement. We argue that p-bits could be used to build energy-efficient probabilistic systems, tailored for probabilistic algorithms and applications. From hardware, architecture, and algorithmic perspectives, we outline the main applications of probabilistic computers ranging from probabilistic machine learning and AI to combinatorial optimization and quantum simulation. Combining emerging nanodevices with the existing CMOS ecosystem will lead to probabilistic computers with orders of magnitude improvements in energy efficiency and probabilistic sampling, potentially unlocking previously unexplored regimes for powerful probabilistic algorithms.
Abstract In-sensor computing (ISC) integrates sensing, memory, and processing at the point of data acquisition, enabling real-time, low-power operation. Two-dimensional (2D) materials offer unique advantages for ISC due to their atomic thickness and multifunctional properties. This review highlights 2D material-based ISC devices, covering mechanisms, performance, and architectures, and discusses challenges and solutions toward scalable fabrication and practical deployment in emerging technologies like Internet of Things (IoT), analog computing, and motion detection.
Quantum Computing is a technology, which promises to overcome the drawbacks of conventional CMOS technology for high density and high performance applications. Its potential to revolutionize today's computing world is attracting more and more researchers towards this field. However, due to the involvement of quantum properties, many beginners find it difficult to follow the field. Therefore, in this research note an effort has been made to introduce the various aspects of quantum computing to researchers, quantum engineers and scientists. The historical background and basic concepts necessary to understand quantum computation and information processing have been introduced in a lucid manner. Various physical implementations and potential application areas of quantum computation have also been discussed in this paper. Recent developments in each realization, in the context of the DiVincenzo criteria, including ion traps based quantum computing, superconducting quantum computing, nuclear magnetic resonance (NMR) quantum computing, spintronics and semiconductor based quantum computing have been discussed.
Dissipation induced by interactions with an external environment typically hinders the performance of quantum computation, but in some cases can be turned out as a useful resource. We show the potential enhancement induced by dissipation in the field of quantum reservoir computing introducing tunable local losses in spin network models. Our approach based on continuous dissipation is able not only to reproduce the dynamics of previous proposals of quantum reservoir computing, based on discontinuous erasing maps but also to enhance their performance. Control of the damping rates is shown to boost popular machine learning temporal tasks as the capability to linearly and non-linearly process the input history and to forecast chaotic series. Finally, we formally prove that, under non-restrictive conditions, our dissipative models form a universal class for reservoir computing. It means that considering our approach, it is possible to approximate any fading memory map with arbitrary precision.
Abstract Neuromorphic computing offers the opportunity to curtail the huge energy demands of modern artificial intelligence (AI) applications by implementing computations into new, brain‐inspired computing architectures. However, the lack of fabrication processes able to integrate several computing units into monolithic systems and the need for new, hardware‐tailored training algorithms still limit the scope of application and performance of neuromorphic hardware. Recent advancements in the field of organic transistors present new opportunities for neuromorphic systems and smart sensing applications, thanks to their unique properties such as neuromorphic behavior, low‐voltage operation, and mixed ionic‐electronic conductivity. Organic neuromorphic transistors push the boundaries of energy efficient brain‐inspired hardware AI, facilitating decentralized on‐chip learning and serving as a foundation for the advancement of closed‐loop intelligent systems in the next generation. The biocompatibility and dual ionic‐electronic conductivity of organic materials introduce new prospects for biointegration and bioelectronics. Their ability to sense and regulate biosystems, as well as their neuro‐inspired functions can be combined with neuromorphic computing to create the next‐generation of bioelectronics. These systems will be able to seamlessly interact with biological systems and locally compute biosignals in a relevant matter.
Abstract Based on first-principles calculations, we demonstrate that 1H/2H-phase transition metal dichalcogenides M X 2 ( M = Nb, Ta; X = S, Se, Te) are unconventional metals, which have an empty-site band of $${A}_{1}^{{\prime} }@1e$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msubsup> <mml:mrow> <mml:mi>A</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>1</mml:mn> </mml:mrow> <mml:mrow> <mml:mo>′</mml:mo> </mml:mrow> </mml:msubsup> <mml:mi>@</mml:mi> <mml:mn>1</mml:mn> <mml:mi>e</mml:mi> </mml:mrow> </mml:math> elementary band representation at the Fermi level. The computed phonon dispersions indicate the stability of the system at high temperatures, while the presence of the soft phonon mode suggests a phase transition to the charge density wave state at low temperatures. Based on the Bardeen-Cooper-Schrieffer theory and computed electron-phonon coupling, our calculations show that the superconductivity (SC) in NbSe 2 is mainly attributed to the soft phonon mode due to the half filling of the empty-site band. Accordingly, the SC has been predicted in unconventional metals TaNS monolayer and 2H-TaN 2 bulk with computed T C = 10 K and 26 K respectively. These results demonstrate that the unconventional metals with partial filling of the empty-site band offer an attractive platform to search for superconductors.
Abstract Majorana fermions are spin-1/2 neutral particles that are their own antiparticles; they were initially predicted by Ettore Majorana in particle physics but their observation still remains elusive. The concept of Majorana fermions has been borrowed by condensed matter physics, where, unlike particle physics, Majorana fermions emerge as zero-energy quasiparticles that can be engineered by combining electrons and holes and have therefore been called Majorana zero modes. In this review, we provide a pedagogical explanation of the basic properties of Majorana zero modes in unconventional superconductors and their consequences in experimental observables, putting a special emphasis on the initial theoretical discoveries. In particular, we first show that Majorana zero modes are self-conjugated and emerge as a special type of zero-energy surface Andreev bound states at the boundary of unconventional superconductors. We then explore Majorana zero modes in 1D spin-polarized p-wave superconductors, where we address the formation of topological superconductivity and the physical realization in superconductor–semiconductor hybrids. In this part we highlight that Majorana quasiparticles appear as zero-energy edge states, exhibiting charge neutrality, spin-polarization, and spatial nonlocality as unique properties that can already be seen from their energies and wavefunctions. Next, we discuss the analytically obtained Green’s functions of p-wave superconductors and demonstrate that the emergence of Majorana zero modes is always accompanied by the formation of odd-frequency spin-triplet pairing as a unique result of the self-conjugate nature of Majorana zero modes. We finally address the signatures of Majorana zero modes in tunneling spectroscopy, including the anomalous proximity effect, and the phase-biased Josephson effect.
Abstract The next generation of soft electronics will expand to the third dimension. This will require the integration of mechanically compliant 3D functional structures with stretchable materials. Here, omnidirectional direct ink writing (DIW) of poly(3,4‐ethylenedioxythiophene): polystyrene sulfonate (PEDOT:PSS) aerogels with tunable electrical and mechanical performance is demonstrated, which can be integrated with soft substrates. Several PEDOT:PSS hydrogels are formulated for DIW and freeze‐dried directly on stretchable substrates to form integrated aerogels displaying high shape fidelity and minimal shrinkage. This technology demonstrates 3D‐structured stretchable interconnects, planar thermoelectric generators for skin electronics, and vertically printed high aspect ratio thermoelectric pillars with ultralow thermal conductivity of 0.065 W m −1 K −1 . The aerogel pillars outpower their dense counterparts in realistic energy harvesting scenarios, where contact resistances cannot be ignored and produced up to 26 nW cm −2 (corresponding to a gravimetric power density of 0.76 mW kg −1 ) for a difference of temperature of 15 K. Here, promising advancements in soft and energy‐efficiency electronic systems relevant to soft robotics and wearables are suggested.
Abstract We present the first investigation of unusual nonlinear Hall effects in twisted multilayer 2D materials. Contrary to expectations, our study shows that these nonlinear effects are not merely extensions of their monolayer counterparts. Instead, we find that stacking order and pairwise interactions between neighboring layers, mediated by Berry curvatures, play a pivotal role in shaping their collective nonlinear optical response. By combining large-scale Real-Time Time-Dependent Density Functional Theory (RT-TDDFT) simulations with model Hamiltonian analyses, we demonstrate a remarkable second-harmonic transverse response in hexagonal boron nitride four-layers, even in cases where the total Berry curvature cancels out. Furthermore, our symmetry analysis of the layered structures provides a simplified framework for predicting nonlinear responses in multilayer materials in general. Our investigation challenges the prevailing understanding of nonlinear optical responses in layered materials and opens new avenues for the design and development of advanced materials with tailored optical properties.
CeSiI has been recently isolated in the ultrathin limit, establishing CeSiI as the first intrinsic two-dimensional van der Waals heavy-fermion material up to 85 K. We show that, due to the strong spin-orbit coupling, the local moments develop a multipolar real-space magnetic texture, leading to local pseudospins with a nearly vanishing net moment. To elucidate its Kondo-screened regime, we extract from first-principles the parameters of the Kondo lattice model describing this material. We develop a pseudofermion methodology in combination with ab initio calculations to reveal the nature of the heavy-fermion state in CeSiI. We analyze the competing magnetic interactions leading to an unconventional heavy-fermion order as a function of the magnetic exchange between the localized f-electrons and the strength of the Kondo coupling. Our results show that the magnetic exchange interactions promote an unconventional momentum-dependent Kondo-screened phase, establishing the nature of the heavy-fermion state observed in CeSiI.
Networks of coupled oscillators have far-reaching implications across various fields, providing insights into a plethora of dynamics. This review offers an in-depth overview of computing with oscillators covering computational capability, synchronization occurrence and mathematical formalism. We discuss numerous circuit design implementations, technology choices and applications from pattern retrieval, combinatorial optimization problems to machine learning algorithms. We also outline perspectives to broaden the applications and mathematical understanding of coupled oscillator dynamics.
Abstract High-temperature unconventional superconductivity quite generically emerges from doping a strongly correlated parent compound, often (close to) an antiferromagnetic insulator. The recently developed dynamical vertex approximation is a state-of-the-art technique that has quantitatively predicted the superconducting dome of nickelates. Here, we apply it to study the effect of pressure in the infinite-layer nickelate Sr x Pr 1− x NiO 2 . We reproduce the increase of the critical temperature ( T c ) under pressure found in experiment up to 12 GPa. According to our results, T c can be further increased with higher pressures. Even without Sr-doping the parent compound, PrNiO 2 , will become a high-temperature superconductor thanks to a strongly enhanced self-doping of the Ni $${d}_{{x}^{2}-{y}^{2}}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mrow> <mml:mi>d</mml:mi> </mml:mrow> <mml:mrow> <mml:msup> <mml:mrow> <mml:mi>x</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> </mml:msup> <mml:mo>−</mml:mo> <mml:msup> <mml:mrow> <mml:mi>y</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> </mml:msup> </mml:mrow> </mml:msub> </mml:math> orbital under pressure. With a maximal T c of 100 K around 100 GPa, nickelate superconductors can reach that of the best cuprates.
Abstract Angle‐resolved spin‐torque ferromagnetic resonance measurements are carried out in heterostructures consisting of Py (Ni 81 Fe 19 ) and a noncollinear antiferromagnetic quantum material IrMn 3 . The structural characterization reveals that IrMn 3 is polycrystalline in nature. A large exchange bias of 158 Oe is found in Py/IrMn 3 at room temperature, while IrMn 3 /Py and Py/Cu/IrMn 3 exhibit no exchange bias. Regardless of the exchange bias and stacking sequence, a substantial unconventional out‐of‐plane anti‐damping torque is observed when IrMn 3 is in direct contact with Py. The magnitude of the out‐of‐plane spin‐orbit torque efficiency is found to be twice as large as the in‐plane spin‐orbit torque efficiency. The unconventional spin‐orbit torque vanishes when a Cu spacer is introduced between Py and IrMn 3 , indicating that the unconventional spin‐orbit torque in this system originates at the interface. These findings are important for realizing efficient antiferromagnet‐based spintronic devices via interfacial engineering.
We present a new scheme for Majorana modes in systems with nonsymmorphic-symmetry-protected band degeneracy. We reveal that when the gapless fermionic excitations are encoded with conventional superconductivity and magnetism, which can be intrinsic or induced by proximity effect, topological superconductivity and Majorana modes can be obtained. We illustrate this outcome in a system which respects the space group P4/nmm and features a fourfold-degenerate fermionic mode at (π, π) in the Brillouin zone. We show that in the presence of conventional superconductivity, different types of topological superconductivity, i.e., first-order and second-order topological superconductivity, with coexisting fragile Wannier obstruction in the latter case, can be generated in accordance with the different types of magnetic orders; Majorana modes are shown to exist on the boundary, at the corner and in the vortices. To further demonstrate the effectiveness of our approach, another example related to the space group P4/ncc based on this scheme is also provided. Our study offers insights into constructing topological superconductors based on bulk energy bands and conventional superconductivity and helps to find new material candidates and design new platforms for realizing Majorana modes. Topological superconductors are highly sought-after systems with potential applications in topological quantum computing. Here, the authors propose a scheme for realizing topological superconductivity based on the bulk energy bands and conventional superconductivity.
Charge-order states of broken symmetry, such as charge density wave (CDW), are able to induce exceptional physical properties, however, the precise understanding of the underlying physics is still elusive. Here, we combine fluctuational electrodynamics and density functional theory to reveal an unconventional thermophotonic effect in CDW-bearing TiSe_{2}, referred to as thermophotonic-CDW (tp-CDW). The interplay of plasmon polariton and CDW electron excitations give rise to an anomalous negative temperature dependency in thermal photons transport, offering an intuitive fingerprint for a transformation of the electron order. Additionally, the demonstrated nontrivial features of tp-CDW transition hold promise for a controllable manipulation of heat flow, which could be extensively utilized in various fields such as thermal science and electron dynamics, as well as in next-generation energy devices.
Abstract We analyze superconductivity in a multi-orbital fermionic system near the onset of a nematic order, using doped FeSe as an example. We associate nematicity with spontaneous polarization between d xz and d yz orbitals. We derive pairing interaction, mediated by soft nematic fluctuations, and show that it is attractive, and its strength depends on the position on the Fermi surface. As the consequence, right at the nematic quantum-critical point (QCP), superconducting gap opens up at T c only at special points and extends into finite arcs at T < T c . In between the arcs the Fermi surface remains intact. This leads to highly unconventional behavior of the specific heat, with no jump at T c and seemingly finite offset at T = 0. We discuss gap structure and pairing symmetry away from a QCP and compare nematic and spin-fluctuation scenarios. We apply the results to FeSe 1− x S x and FeSe 1− x Te x .
Simulating fluid dynamics on a quantum computer is intrinsically difficult due to the nonlinear and non-Hamiltonian nature of the Navier-Stokes equation (NSE). We propose a framework for quantum computing of fluid dynamics based on the hydrodynamic Schr\"odinger equation (HSE), which can be promising in simulating three-dimensional turbulent flows in various engineering applications. The HSE is derived by generalizing the Madelung transform to compressible or incompressible flows with finite vorticity and dissipation. Since the HSE is expressed as a unitary operator on a two-component wave function, it is more suitable than the NSE for quantum computing. The flow governed by the HSE can resemble a turbulent flow consisting of tangled vortex tubes with the five-thirds scaling of energy spectrum. We develop a prediction-correction quantum algorithm to solve the HSE. This algorithm is implemented for simple flows on the quantum simulator Qiskit with partial exponential speedup.